"Valencia CF and Martin Montoya have reached an agreement with the player, who joins the club for the next four seasons," Valencia said in a statement on Monday, reports Xinhua.
Montoya entered the first team at the Camp Nou in 2011, but only made 45 La Liga appearances for Barca in five seasons.
The 25-year-old Spaniard was loaned to Inter Milan and Real Betis last season.
Valencia got a disappointing finish of 12th place in La Liga last season.
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